Easy interpretation of optical two-dimensional correlation spectra

Opt Lett. 2006 Nov 15;31(22):3354-6. doi: 10.1364/ol.31.003354.

Abstract

We demonstrate that the value of the underlying frequency-frequency correlation function can be retrieved from a two-dimensional optical correlation spectrum through a simple relationship. The proposed method yields both intuitive clues and a quantitative measure of the dynamics of the system. The technique is applied to studying the effects of temperature and phase changes on liquid-glass solvent dynamics.